Bio-Inspired NanoVilli Chips for Enhanced Capture of Tumor-Derived Extracellular Vesicles: Toward Non-Invasive Detection of Gene Alterations in Non-Small Cell Lung Cancer

ACS Appl Mater Interfaces. 2019 Apr 17;11(15):13973-13983. doi: 10.1021/acsami.9b01406. Epub 2019 Apr 2.

Abstract

Tumor-derived extracellular vesicles (EVs) present in bodily fluids are emerging liquid biopsy markers for non-invasive cancer diagnosis and treatment monitoring. Because the majority of EVs in circulation are not of tumor origin, it is critical to develop new platforms capable of enriching tumor-derived EVs from the blood. Herein, we introduce a biostructure-inspired NanoVilli Chip, capable of highly efficient and reproducible immunoaffinity capture of tumor-derived EVs from blood plasma samples. Anti-EpCAM-grafted silicon nanowire arrays were engineered to mimic the distinctive structures of intestinal microvilli, dramatically increasing surface area and enhancing tumor-derived EV capture. RNA in the captured EVs can be recovered for downstream molecular analyses by reverse transcription Droplet Digital PCR. We demonstrate that this assay can be applied to monitor the dynamic changes of ROS1 rearrangements and epidermal growth factor receptor T790M mutations that predict treatment responses and disease progression in non-small cell lung cancer patients.

Keywords: EGFR T790M mutation; ROS1 rearrangements; extracellular vesicles; microfluidics; nanosubstrates; non-small cell lung cancer.

MeSH terms

  • Adult
  • Aged
  • Antibodies, Immobilized / chemistry
  • Antibodies, Immobilized / immunology
  • Biomarkers, Tumor / genetics
  • Carcinoma, Non-Small-Cell Lung / genetics
  • Carcinoma, Non-Small-Cell Lung / pathology*
  • Epithelial Cell Adhesion Molecule / immunology
  • ErbB Receptors / genetics*
  • Extracellular Vesicles / metabolism*
  • Female
  • Gene Rearrangement
  • Humans
  • Lung Neoplasms / genetics
  • Lung Neoplasms / pathology*
  • Male
  • Middle Aged
  • Nanowires / chemistry*
  • Polymerase Chain Reaction
  • Polymorphism, Single Nucleotide
  • Protein-Tyrosine Kinases / genetics*
  • Proto-Oncogene Proteins / genetics*
  • RNA, Messenger / metabolism
  • Silicon / chemistry

Substances

  • Antibodies, Immobilized
  • Biomarkers, Tumor
  • Epithelial Cell Adhesion Molecule
  • Proto-Oncogene Proteins
  • RNA, Messenger
  • ErbB Receptors
  • Protein-Tyrosine Kinases
  • ROS1 protein, human
  • Silicon