Molecular modeling and biological studies show that some μ-opioid receptor agonists might elicit analgesia acting as MMP-9 inhibitors

Future Med Chem. 2019 Jun;11(11):1245-1258. doi: 10.4155/fmc-2018-0535. Epub 2019 Apr 12.

Abstract

Aim: Despite the serious side effects, analgesics acting on opioid receptors are still considered the best way to get antinociception. Matrix metalloproteinases, a large family of zinc-dependent proteases implicated in many pathological conditions, such as diabetes and osteoarthritis, are also involved in inflammation and pain. Methodology & results: Looking for evidence of possible interactions of opioid pathways and inflammation mediators, molecular modeling studies of a series of recently developed μ-opioid receptor benzomorphanic agonists together with biological data on pain and inflammation molecular targets, allowed us to hypothesize a possible correlation between μ-opioid receptor system and MMP-9. Conclusion: A new compound, (-)-MML1017, emerged as a possible dual-acting agent able to interact selectively and potently with the two molecular targets.

Keywords: MMP-9 inhibitors; MOR agonists; drug discovery; inflammation; molecular modeling; multitarget drugs; pain.

Publication types

  • Research Support, Non-U.S. Gov't

MeSH terms

  • Analgesics / chemistry
  • Analgesics / pharmacology*
  • Benzomorphans / chemistry
  • Benzomorphans / pharmacology*
  • Drug Discovery
  • HEK293 Cells
  • Humans
  • Matrix Metalloproteinase 9 / chemistry
  • Matrix Metalloproteinase 9 / metabolism*
  • Matrix Metalloproteinase Inhibitors / chemistry
  • Matrix Metalloproteinase Inhibitors / pharmacology*
  • Models, Molecular
  • Receptors, Opioid, mu / agonists*

Substances

  • Analgesics
  • Benzomorphans
  • Matrix Metalloproteinase Inhibitors
  • Receptors, Opioid, mu
  • Matrix Metalloproteinase 9