Improved matrix coating for positive- and negative-ion-mode MALDI-TOF imaging of lipids in blood vessel tissues

Anal Bioanal Chem. 2019 Jun;411(15):3221-3227. doi: 10.1007/s00216-019-01826-x. Epub 2019 Apr 30.

Abstract

High-quality matrix-assisted laser desorption/ionization mass spectrometry imaging (MALDI MSI) of lipids in biological tissue relies on the fabrication of a homogeneous matrix coating featuring best possible analyte integration. This communication addresses a matrix vapor deposition/recrystallization process for the application of 1,5-diaminonaphthalene (1,5-DAN) onto slices of human aortic tissue. The matrix coating is compatible with both positive- as well as negative-ion-mode MALDI MSI facilitating a significantly enhanced detection of lipid-related signals in different cell layers of blood vessel walls. Graphical abstract.

Keywords: Lipidomics; MALDI MSI; Matrix vapor deposition/recrystallization; Thoracic aortic aneurysm.

MeSH terms

  • 2-Naphthylamine / analogs & derivatives
  • 2-Naphthylamine / chemistry
  • Aorta / chemistry*
  • Aorta / ultrastructure
  • Cold Temperature
  • Humans
  • Lipids / analysis*
  • Spectrometry, Mass, Matrix-Assisted Laser Desorption-Ionization / methods*
  • Staining and Labeling
  • Vacuum

Substances

  • Lipids
  • 1,5-diaminonaphthalene
  • 2-Naphthylamine