Bio-orthogonal chemistry-based method for fluorescent labelling of ribosomal RNA in live mammalian cells

Chem Commun (Camb). 2019 Aug 27;55(70):10456-10459. doi: 10.1039/c9cc05346h.

Abstract

A bio-orthogonal chemistry-based approach for fluorescent labelling of ribosomal RNA is described. It involves an adenosine analogue modified with trans-cyclooctene and masked 5'-phosphate group using aryl phosphoramidate. The incorporation into rRNA has been confirmed using agarose gel electrophoresis, as well as a highly sensitive UHPLC-MS/MS method. Fluorescent labelling of rRNA has been achieved in live HeLa cells via an inverse electron demand Diels-Alder reaction with a tetrazine conjugated to an Oregon Green fluorophore. This communication describes the stepwise approach that led to the development and characterization of the probe. The results demonstrate a new strategy towards development of future fluorescent probes to investigate the biochemistry of nucleic acids.

MeSH terms

  • Chromatography, High Pressure Liquid / methods
  • Cycloaddition Reaction
  • Fluorescent Dyes / chemistry*
  • HeLa Cells
  • Humans
  • RNA, Ribosomal / chemistry*
  • Tandem Mass Spectrometry / methods

Substances

  • Fluorescent Dyes
  • RNA, Ribosomal