In vitro prenatal developmental toxicity induced by some petroleum substances is mediated by their 3- to 7-ring PAH constituent with a potential role for the aryl hydrocarbon receptor (AhR)

Toxicol Lett. 2019 Oct 15:315:64-76. doi: 10.1016/j.toxlet.2019.08.001. Epub 2019 Aug 13.

Abstract

To test the hypothesis that 3-7 ring polycyclic aromatic hydrocarbons (PAHs) are responsible for the prenatal developmental toxicity (PDT) as observed with some petroleum substances (PS), the present study evaluates the PDT potency of DMSO-extracts of 7 heavy fuel oils (HFO), varying in their PAH content, and 1 highly refined base oil (HRBO), containing no aromatics, in the embryonic stem cell test (EST). All DMSO-extracts of HFO inhibit ES-D3 cell differentiation in a concentration-dependent manner and their potency is proportional to the amount of 3-7 ring PAHs they contain. All DMSO-extracts of HFOs also show aryl hydrocarbon receptor (AhR)-mediated activities, as tested in the AhR-CALUX assay. Contrarily, the HRBO-extract tested negative in both assays. Co-exposure of ES-D3 cells with selected DMSO-extracts of PS and the AhR-antagonist trimethoxyflavone, successfully counteracted the PS-induced inhibition of ES-D3 cell differentiation, confirming the role of the AhR in mediating the observed PDT of PS extracts in the EST. A good correlation exists when comparing the in-vitro with the in-vivo PDT potencies of the PS under study. Altogether, our findings corroborate the hypothesis that PS-induced PDT is caused by 3-7 ring PAHs present in these substances and that the observed PDT is partially AhR-mediated.

Keywords: Aryl hydrocarbon receptor; Embryonic stem cell test; Petroleum substances; Polycyclic aromatic hydrocarbons; Prenatal developmental toxicity; UVCBs.

MeSH terms

  • Biological Assay
  • Embryonic Stem Cells / drug effects*
  • Environmental Pollutants / metabolism
  • Environmental Pollutants / toxicity*
  • Female
  • Humans
  • Petroleum / metabolism
  • Petroleum / toxicity*
  • Polycyclic Aromatic Hydrocarbons / metabolism*
  • Polycyclic Aromatic Hydrocarbons / toxicity*
  • Pregnancy
  • Prenatal Exposure Delayed Effects / chemically induced*
  • Receptors, Aryl Hydrocarbon / metabolism*

Substances

  • Environmental Pollutants
  • Petroleum
  • Polycyclic Aromatic Hydrocarbons
  • Receptors, Aryl Hydrocarbon