Influence of sediment parameters on the distribution and fate of PAHs in an estuarine tropical region located in the Brazilian semi-arid (Jaguaribe River, Ceará coast)

Mar Pollut Bull. 2019 Sep:146:703-710. doi: 10.1016/j.marpolbul.2019.07.027. Epub 2019 Jul 19.

Abstract

18 polycyclic aromatic hydrocarbons (PAHs) were evaluated in the Jaguaribe River to explore the influence of grain size, organic carbon, humic and fulvic acids and black carbon on their adsorption onto sediment. The ∑PAHs concentrations variated from 0.6 to 3752.0 ng g-1 with highest concentrations in the estuarine zone. The PAHs predominant source along the river was from mixed sources, mainly related to biomass combustion, small oil spills related to recreational nautical activities and runoff from cities. Organic and inorganic parameters presented influence on PAHs distribution along the river, with humic acid as a determinant factor. These research findings are of importance to an assessment of the fate and transport of PAHs in estuarine systems.

Keywords: Black carbon; Fate and transport; Humic and fulvic acid; Jaguaribe River; Organic matter; PAHs.

MeSH terms

  • Brazil
  • Cities
  • Environmental Monitoring
  • Geologic Sediments / analysis
  • Geologic Sediments / chemistry*
  • Humic Substances / analysis
  • Polycyclic Aromatic Hydrocarbons / analysis*
  • Rivers / chemistry
  • Tropical Climate
  • Water Pollutants, Chemical / analysis*
  • Wetlands

Substances

  • Humic Substances
  • Polycyclic Aromatic Hydrocarbons
  • Water Pollutants, Chemical