Cyclin dependent kinase (CDK) inhibitors as anticancer drugs: Recent advances (2015-2019)

Bioorg Med Chem Lett. 2019 Oct 15;29(20):126637. doi: 10.1016/j.bmcl.2019.126637. Epub 2019 Aug 26.

Abstract

Sustained proliferative capacity and gene dysregulation are hallmarks of cancer. In mammalian cells, cyclin-dependent kinases (CDKs) control critical cell cycle checkpoints and key transcriptional events in response to extracellular and intracellular signals leading to proliferation. Significant clinical activity for the treatment of hormone receptor positive metastatic breast cancer has been demonstrated by palbociclib, ribociclib and abemaciclib, dual CDK4/6 inhibitors recently FDA-approved. SY-1365, a CDK7 inhibitor has shown initial encouraging data in phase I for solid tumors treatment. These results have rejuvenated the CDKs research field. This review provides an overview of relevant advances on CDK inhibitor research since 2015 to 2019, with special emphasis on transcriptional CDK inhibitors, new emerging strategies such as target protein degradation and compounds under clinical evaluation.

Keywords: CDK degradation; CDK inhibitors; Cell cycle; Covalent inhibitors; Transcription.

Publication types

  • Research Support, Non-U.S. Gov't
  • Review

MeSH terms

  • Aminopyridines / chemistry
  • Aminopyridines / pharmacology
  • Animals
  • Antineoplastic Agents / chemistry*
  • Antineoplastic Agents / pharmacology
  • Benzimidazoles / chemistry
  • Benzimidazoles / pharmacology
  • Breast Neoplasms / drug therapy*
  • Cell Cycle Checkpoints / drug effects
  • Cyclin-Dependent Kinases / antagonists & inhibitors*
  • Drug Discovery
  • Humans
  • Indoles / chemistry
  • Indoles / pharmacology
  • Piperazines / chemistry
  • Piperazines / pharmacology
  • Protein Kinase Inhibitors / chemistry*
  • Protein Kinase Inhibitors / pharmacology
  • Purines / chemistry
  • Purines / pharmacology
  • Pyridines / chemistry*
  • Pyridines / pharmacology
  • Pyrimidines / chemistry*
  • Pyrimidines / pharmacology
  • Transcription Factors / metabolism

Substances

  • Aminopyridines
  • Antineoplastic Agents
  • Benzimidazoles
  • Indoles
  • Piperazines
  • Protein Kinase Inhibitors
  • Purines
  • Pyridines
  • Pyrimidines
  • Transcription Factors
  • abemaciclib
  • mevociclib
  • Cyclin-Dependent Kinases
  • palbociclib
  • ribociclib