ImmunoPET, [64Cu]Cu-DOTA-Anti-CD33 PET-CT, Imaging of an AML Xenograft Model

Clin Cancer Res. 2019 Dec 15;25(24):7463-7474. doi: 10.1158/1078-0432.CCR-19-1106. Epub 2019 Sep 23.

Abstract

Purpose: Acute myeloid leukemia (AML) is a highly aggressive form of leukemia, which results in poor survival outcomes. Currently, diagnosis and prognosis are based on invasive single-point bone marrow biopsies (iliac crest). There is currently no AML-specific noninvasive imaging method to detect disease, including in extramedullary organs, representing an unmet clinical need. About 85% to 90% of human myeloid leukemia cells express CD33 cell surface receptors, highlighting CD33 as an ideal candidate for AML immunoPET.

Experimental design: We evaluated whether [64Cu]Cu-DOTA-anti-CD33 murine mAb can be used for immunoPET imaging of AML in a preclinical model. MicroCT was adjusted to detect spatial/anatomical details of PET activity. For translational purposes, a humanized anti-CD33 antibody was produced; we confirmed its ability to detect disease and its distribution. We reconfirmed/validated CD33 antibody-specific targeting with an antibody-drug conjugate (ADC) and radioimmunotherapy (RIT).

Results: [64Cu]Cu-DOTA-anti-CD33-based PET-CT imaging detected CD33+ AML in mice with high sensitivity (95.65%) and specificity (100%). The CD33+ PET activity was significantly higher in specific skeletal niches [femur (P < 0.00001), tibia (P = 0.0001), humerus (P = 0.0014), and lumber spine (P < 0.00001)] in AML-bearing mice (over nonleukemic control mice). Interestingly, the hybrid PET-CT imaging showed high disease activity in the epiphysis/metaphysis of the femur, indicating regional spatial heterogeneity. Anti-CD33 therapy using newly developed humanized anti-CD33 mAb as an ADC (P = 0.02) and [225Ac]Ac-anti-CD33-RIT (P < 0.00001) significantly reduced disease burden over that of respective controls.

Conclusions: We have successfully developed a novel anti-CD33 immunoPET-CT-based noninvasive modality for AML and its spatial distribution, indicating a preferential skeletal niche.

Publication types

  • Research Support, N.I.H., Extramural

MeSH terms

  • Animals
  • Antibodies, Monoclonal, Humanized / pharmacokinetics
  • Cell Line, Tumor
  • Copper Radioisotopes / chemistry*
  • Disease Models, Animal
  • Heterocyclic Compounds, 1-Ring / chemistry*
  • Immunoconjugates / pharmacokinetics*
  • Leukemia, Myeloid, Acute / diagnostic imaging*
  • Leukemia, Myeloid, Acute / drug therapy
  • Leukemia, Myeloid, Acute / pathology
  • Mice
  • Mice, Inbred NOD
  • Mice, SCID
  • Positron Emission Tomography Computed Tomography / methods*
  • Radiopharmaceuticals / pharmacokinetics*
  • Sialic Acid Binding Ig-like Lectin 3 / antagonists & inhibitors
  • Sialic Acid Binding Ig-like Lectin 3 / immunology*
  • Tissue Distribution
  • Xenograft Model Antitumor Assays

Substances

  • Antibodies, Monoclonal, Humanized
  • CD33 protein, human
  • Copper Radioisotopes
  • Heterocyclic Compounds, 1-Ring
  • Immunoconjugates
  • Radiopharmaceuticals
  • Sialic Acid Binding Ig-like Lectin 3
  • 1,4,7,10-tetraazacyclododecane- 1,4,7,10-tetraacetic acid