Identification and characterization of a novel bacterial carbohydrate esterase from the bacterium Pantoea ananatis Sd-1 with potential for degradation of lignocellulose and pesticides

Biotechnol Lett. 2020 Aug;42(8):1479-1488. doi: 10.1007/s10529-020-02855-8. Epub 2020 Mar 6.

Abstract

Objective: Identification and characterization of a novel bacterial carbohydrate esterase (PaCes7) with application potential for lignocellulose and pesticide degradation.

Results: PaCes7 was identified from the lignocellulolytic bacterium, Pantoea ananatis Sd-1 as a new carbohydrate esterase. Recombinant PaCes7 heterologously expressed in Escherichia coli showed a clear preference for esters with short-chain fatty acids and exhibited maximum activity towards α-naphthol acetate at 37 °C and pH 7.5. Purified PaCes7 exhibited its catalytic activity under mesophilic conditions and retained more than 40% activity below 30 °C. It displayed a relatively wide pH stability from pH 6-11. Furthermore, the enzyme was strongly resistant to Mg2+, Pb2+, and Co2+ and activated by K+ and Ca2+. Both P. ananatis Sd-1 and PaCes7 could degrade the pesticide carbaryl. Additionally, PaCes7 was shown to work in combination with cellulase and/or xylanase in rice straw degradation.

Conclusions: The data suggest that PaCes7 possesses promising biotechnological potential.

Keywords: Carbaryl; Carbohydrate esterase; Degradation; Lignocellulose; Pantoea ananatis.

MeSH terms

  • Bacterial Proteins* / chemistry
  • Bacterial Proteins* / genetics
  • Bacterial Proteins* / metabolism
  • Biodegradation, Environmental
  • Carbaryl / metabolism
  • Enzyme Stability
  • Esterases* / chemistry
  • Esterases* / genetics
  • Esterases* / metabolism
  • Lignin / metabolism*
  • Pantoea / enzymology*
  • Pantoea / genetics
  • Pesticides / metabolism*

Substances

  • Bacterial Proteins
  • Pesticides
  • lignocellulose
  • Lignin
  • Esterases
  • Carbaryl

Supplementary concepts

  • Pantoea ananatis