Simultaneous determination of canrenone, digoxin and tolvaptan by UHPLC-MS/MS: application in heart failure patients

Bioanalysis. 2020 May;12(9):569-582. doi: 10.4155/bio-2020-0037. Epub 2020 May 29.

Abstract

Aim: Heart failure patients are frequently given comedication of digoxin and diuretics like spironolactone and tolvaptan. A UHPLC-MS/MS assay for determining canrenone (main active metabolite of spironolactone), digoxin and tolvaptan simultaneously should be developed so as to support related drug-drug interaction studies. Results: A UHPLC-MS/MS method for simultaneous determination of these three drugs in human plasma was established and fully verified as per CFDA guidelines. Chromatographic separation was achieved using a 4-min isocratic elution. Mass analyses were performed under positive electrospray ionization mode. The calibration curves were established over 1.0-400.0 ng/ml for canrenone and tolvaptan while over 0.1-40.0 ng/ml for digoxin. Conclusion: The developed method was feasible in detecting concentration and related drug-drug interaction studies.

Keywords: UHPLC–MS/MS; canrenone; digoxin; drug–drug interactions; heart failure; tolvaptan.

MeSH terms

  • Canrenone / blood*
  • Chromatography, High Pressure Liquid
  • Digoxin / blood*
  • Heart Failure / blood*
  • Humans
  • Tandem Mass Spectrometry
  • Tolvaptan / blood*

Substances

  • Tolvaptan
  • Digoxin
  • Canrenone