Tarragon essential oil as a source of bioactive compounds with anti-quorum sensing and anti-proteolytic activity against Pseudomonas spp. isolated from fish - in vitro, in silico and in situ approaches

Int J Food Microbiol. 2020 Oct 16:331:108732. doi: 10.1016/j.ijfoodmicro.2020.108732. Epub 2020 Jun 5.

Abstract

The present study aimed to evaluate the anti-quorum sensing (anti-QS) and anti-proteolytic potentials of tarragon essential oil (TEO) and its major compounds against food-associated Pseudomonas spp. The activities were verified by in vitro, in silico and in situ approaches. In this work, methyl eugenol (ME)- and β-phellandrene (β-PH)-rich TEO was investigated. TEO at subMIC increased the percentage of saturated fatty acids in the bacterial membranes (from 7 to 22%) and exhibited anti-quorum sensing via decreasing the efficiency of QS autoinducer synthesis [3-oxo-C12-HSL (from 2.028 μg/mL to <LOD), C4-HSL (from 1.312 μg/mL to <LOD) and PQS (from 0.007625 μg/mL to <LOD)]. ME and β-PH were docked into LasR, RhlR and PqsR proteins, with docking scores comparable to native autoinductors. The subMICs of TEO, ME and β-PH decreased the proteolysis in the examined bacteria by 33, 29, and 21% (in TSB medium) and by 29, 26, and 19% (in fish juice medium), respectively. Almost all genes encoding proteases were downregulated by the applied agents. The ME- and β-PH-rich TEO acts as an anti-QS agent and significantly suppresses the proteolytic activity of food-associated pseudomonads. It might therefore increase the quality of fish-based products, where Pseudomonas spp. predominate.

Keywords: Autoinductors; Food spoilage; Gene expression; Molecular docking; subMIC.

MeSH terms

  • 4-Butyrolactone / analogs & derivatives
  • 4-Butyrolactone / isolation & purification
  • 4-Butyrolactone / pharmacology
  • Animals
  • Anti-Bacterial Agents / isolation & purification
  • Anti-Bacterial Agents / pharmacology
  • Artemisia / chemistry*
  • Computer Simulation
  • Fishes / microbiology
  • Homoserine / analogs & derivatives
  • Homoserine / isolation & purification
  • Homoserine / pharmacology
  • Oils, Volatile / chemistry
  • Oils, Volatile / isolation & purification
  • Oils, Volatile / pharmacology*
  • Proteolysis / drug effects*
  • Pseudomonas / drug effects*
  • Pseudomonas / isolation & purification
  • Quorum Sensing / drug effects*

Substances

  • Anti-Bacterial Agents
  • N-(3-oxododecanoyl)homoserine lactone
  • N-butyrylhomoserine lactone
  • Oils, Volatile
  • Homoserine
  • 4-Butyrolactone