Structural characterization and effect on leukopenia of fucoidan from Durvillaea antarctica

Carbohydr Polym. 2021 Mar 15:256:117529. doi: 10.1016/j.carbpol.2020.117529. Epub 2020 Dec 17.

Abstract

Fucoidans from brown seaweed shows various bioactive properties and promising prospects in biomedical field. Here, a novel fucoidan (F-4) was extracted and purified from Durvillaea antarctica. The structure of F-4 was characterized by HPLC, HPGPC, GC-MS, together with IR and NMR spectral analysis. F-4 is a sulfated polysaccharide mainly composed of fucose (Fuc), galactose (Gal), and glucose (Glc) in a molar ratio of 26.4: 7.1: 1.0. The backbone of F-4 is composed of (1→3) and (1→4)-linked-α-L-Fucp residues, which sulfated at C-4 or C-2 positions and branched with α-L-Fuc, β-D-Gal, and β-D-Glc residues. Furthermore, F-4 can effectively promote the growth of leukocyte in a mouse model induced by cyclophosphamide, possibly by activating hematopoietic progenitor cells and regulating the hematopoietic microenvironment of bone marrow. Our data provide useful information for further investigation of fucoidan in the treatment of chemotherapy-induced leukopenia.

Keywords: Durvillaea antarctica; Fucoidan; Leukopenia; Structural characterization.

MeSH terms

  • Animals
  • Antineoplastic Agents / adverse effects
  • Bone Marrow / metabolism
  • Bone Marrow Cells / cytology
  • Cell Proliferation
  • Chromatography, High Pressure Liquid
  • Cyclophosphamide / chemistry
  • DNA / analysis
  • Gas Chromatography-Mass Spectrometry
  • Hematopoietic Stem Cells / cytology
  • Leukocytes / cytology
  • Leukopenia / chemically induced
  • Leukopenia / drug therapy*
  • Magnetic Resonance Spectroscopy
  • Male
  • Methylation
  • Mice
  • Polysaccharides / isolation & purification
  • Polysaccharides / pharmacology*
  • Seaweed / chemistry*
  • Spectrophotometry, Infrared
  • Spectroscopy, Fourier Transform Infrared
  • Stromal Cells / cytology

Substances

  • Antineoplastic Agents
  • Polysaccharides
  • Cyclophosphamide
  • DNA
  • fucoidan