Total Synthesis of ent-Plagiochianin B

Org Lett. 2021 Feb 19;23(4):1243-1246. doi: 10.1021/acs.orglett.0c04219. Epub 2021 Jan 30.

Abstract

An enantioselective total synthesis of plagiochianin B is described that employs (+)-3-carene as its point of departure and delivers the enantiomer of the natural product. Key features of the synthesis include a palladium-mediated regioselective oxidative cleavage of an olefin residing on a pyridine derived from a 6π-azatriene electrocyclization.

Publication types

  • Research Support, N.I.H., Extramural
  • Research Support, Non-U.S. Gov't

MeSH terms

  • Alkenes / chemistry*
  • Biological Products
  • Cyclization
  • Molecular Structure
  • Palladium / chemistry*
  • Stereoisomerism

Substances

  • Alkenes
  • Biological Products
  • Palladium