Total synthesis of (-)-cephalosporolide D

Nat Prod Res. 2022 Aug;36(15):4021-4025. doi: 10.1080/14786419.2021.1896509. Epub 2021 Mar 15.

Abstract

In this communication, a concise and efficient synthetic route for the synthesis of (-)-Cephalosporolide D in enantioselective way has been described. In this synthesis, Mitsunobu esterification and Ring Closing Metathesis (RCM) for macrocyclic ring formation have been applied as key steps.

Keywords: (–)-Cephalosporolide D; Barbier allylation; Mitsunobu esterification; Ring Closing Metathesis (RCM).

MeSH terms

  • Cyclization
  • Lactones*

Substances

  • Lactones
  • cephalosporolide D