Rapid 18F-labeling via Pd-catalyzed S-arylation in aqueous medium

Chem Commun (Camb). 2021 Apr 14;57(29):3547-3550. doi: 10.1039/d1cc00745a. Epub 2021 Mar 19.

Abstract

We report radiolabeling of thiol-containing substrates via Pd-catalyzed S-arylation with 2-[18F]fluoro-5-iodopyridine, which is readily accessible using the "minimalist" radiofluorination method. The practicality of the procedure was confirmed by preparation of a novel PSMA-specific PET-tracer as well as labeling of glutathione, Aβ oligomer-binding RD2 peptide, bovine serum albumin and PSMA I&S.