Self-Assembly Iron Oxide Nanoclusters for Photothermal-Mediated Synergistic Chemo/Chemodynamic Therapy

J Immunol Res. 2021 Apr 7:2021:9958239. doi: 10.1155/2021/9958239. eCollection 2021.

Abstract

Methods: Superparamagnetic iron oxide nanoclusters (SPIOCs) were located within the core, which resulted in high photothermal conversion and outstanding generation of reactive oxygen species (ROS). The shell consisted of a human serum albumin- (HSA-) paclitaxel (PTX) layer, which extended the blood circulation time and ensured the effectiveness of the chemotherapy. Arg-Gly-Asp peptides (RGD) were linked to the naked cysteine moieties in HSA to promote the specific targeting of human glioma U87 cells by α v β 3 integrins. Continuous near-infrared light irradiation triggered and promoted the synergistic chemo/CDT therapy through the photothermal effect.

Results: Our SPIOCs@HSA-RGD nanoplatform showed well biocompatibility and could target glioma specifically. Photothermal conversion and ROS burst were detected after continuous 808 nm light irradiation, and a significant antitumor effect was achieved.

Conclusion: Experimental in vitro and in vivo evaluations showed that our photothermal-mediated chemo/CDT therapy could efficiently inhibit tumor growth and is therefore promising for cancer therapy.

MeSH terms

  • Animals
  • Antineoplastic Combined Chemotherapy Protocols / therapeutic use*
  • Cell Growth Processes
  • Cell Line, Tumor
  • Chemoradiotherapy / methods*
  • Drug Synergism
  • Glioma / therapy*
  • Humans
  • Infrared Rays
  • Integrin alphaVbeta3 / metabolism
  • Integrin alphaVbeta3 / therapeutic use*
  • Magnetic Iron Oxide Nanoparticles / administration & dosage
  • Magnetic Iron Oxide Nanoparticles / chemistry
  • Male
  • Mice
  • Mice, Inbred BALB C
  • Mice, Nude
  • Oligopeptides / chemistry
  • Oligopeptides / therapeutic use*
  • Paclitaxel / chemistry
  • Paclitaxel / therapeutic use*
  • Rats
  • Reactive Oxygen Species / metabolism
  • Serum Albumin, Human / chemistry
  • Theranostic Nanomedicine / methods*
  • Xenograft Model Antitumor Assays

Substances

  • Integrin alphaVbeta3
  • Oligopeptides
  • Reactive Oxygen Species
  • arginyl-glycyl-aspartic acid
  • Paclitaxel
  • Serum Albumin, Human