Frequency comb-based multidimensional coherent spectroscopy bridges the gap between fundamental science and cutting-edge technology

J Chem Phys. 2021 Apr 28;154(16):160901. doi: 10.1063/5.0047164.

Abstract

Optical multidimensional coherent spectroscopy (MDCS) has become a powerful and routine technique for studying optical properties of a wide range of materials. However, current implementations of MDCS have spectral resolution and acquisition speed limitations. In this Perspective, I describe how frequency comb technology can be used to overcome the limitations and also show the recent progress that has been made in this field.