Microemulsion for Prolonged Release of Fenretinide in the Mammary Tissue and Prevention of Breast Cancer Development

Mol Pharm. 2021 Sep 6;18(9):3401-3417. doi: 10.1021/acs.molpharmaceut.1c00319. Epub 2021 Aug 17.

Abstract

The need of pharmacological strategies to preclude breast cancer development motivated us to develop a non-aqueous microemulsion (ME) capable of forming a depot after administration in the mammary tissue and uptake of interstitial fluids for prolonged release of the retinoid fenretinide. The selected ME was composed of phosphatidylcholine/tricaprylin/propylene glycol (45:5:50, w/w/w) and presented a droplet diameter of 175.3 ± 8.9 nm. Upon water uptake, the ME transformed successively into a lamellar phase, gel, and a lamellar phase-containing emulsion in vitro as the water content increased and released 30% of fenretinide in vitro after 9 days. Consistent with the slow release, the ME formed a depot in cell cultures and increased fenretinide IC50 values by 68.3- and 13.2-fold in MCF-7 and T-47D cells compared to a solution, respectively. At non-cytotoxic concentrations, the ME reduced T-47D cell migration by 75.9% and spheroid growth, resulting in ∼30% smaller structures. The depot formed in vivo prolonged a fluorochrome release for 30 days without producing any sings of local irritation. In a preclinical model of chemically induced carcinogenesis, ME administration every 3 weeks for 3 months significantly reduced (4.7-fold) the incidence of breast tumors and increased type II collagen expression, which might contribute to limit spreading. These promising results support the potential ME applicability as a preventive therapy of breast cancer.

Keywords: breast cancer; chemoprevention; fenretinide; in situ gelling; microemulsion; sustained release..

Publication types

  • Research Support, Non-U.S. Gov't

MeSH terms

  • Animals
  • Anticarcinogenic Agents / administration & dosage*
  • Anticarcinogenic Agents / pharmacokinetics
  • Breast Neoplasms / chemically induced
  • Breast Neoplasms / pathology
  • Breast Neoplasms / prevention & control*
  • Cell Survival / drug effects
  • Delayed-Action Preparations / administration & dosage
  • Delayed-Action Preparations / pharmacokinetics
  • Drug Liberation
  • Drug Screening Assays, Antitumor
  • Emulsions
  • Female
  • Fenretinide / administration & dosage*
  • Fenretinide / pharmacokinetics
  • Humans
  • Inhibitory Concentration 50
  • MCF-7 Cells
  • Mammary Glands, Animal / drug effects
  • Mammary Glands, Animal / pathology
  • Mammary Neoplasms, Experimental / chemically induced
  • Mammary Neoplasms, Experimental / pathology
  • Mammary Neoplasms, Experimental / prevention & control*
  • Methylnitrosourea / administration & dosage
  • Methylnitrosourea / toxicity
  • Mice
  • Rats

Substances

  • Anticarcinogenic Agents
  • Delayed-Action Preparations
  • Emulsions
  • Fenretinide
  • Methylnitrosourea