A Reference Range for Plasma Levels of Inorganic Pyrophosphate in Children Using the ATP Sulfurylase Method

J Clin Endocrinol Metab. 2022 Jan 1;107(1):109-118. doi: 10.1210/clinem/dgab615.

Abstract

Purpose: Generalized arterial calcification of infancy, pseudoxanthoma elasticum, autosomal recessive hypophosphatemic rickets type 2, and hypophosphatasia are rare inherited disorders associated with altered plasma levels of inorganic pyrophosphate (PPi). In this study, we aimed to establish a reference range for plasma PPi in the pediatric population, which would be essential to support its use as a biomarker in children with mineralization disorders.

Methods: Plasma samples were collected from 200 children aged 1 day to 18 years who underwent blood testing for medical conditions not affecting plasma PPi levels. PPi was measured in proband plasma utilizing a validated adenosine triphosphate (ATP) sulfurylase method.

Results: The analytical sensitivity of the ATP sulfurylase assay consisted of 0.15 to 10 µM PPi. Inter- and intra-assay coefficients of variability on identical samples were below 10%. The standard range of PPi in the blood plasma of children and adolescents aged 0 to 18 years was calculated as 2.36 to 4.44 µM, with a median of 3.17 µM, with no difference between male and female probands. PPi plasma levels did not differ significantly in different pediatric age groups.

Main conclusions: Our results yielded no noteworthy discrepancy to the reported standard range of plasma PPi in adults (2-5 µM). We propose the described ATP sulfurylase method as a diagnostic tool to measure PPi levels in plasma as a biomarker in the pediatric population.

Keywords: ABCC6; ATP sulfurylase assay; ENPP1; autosomal recessive hypophosphatemic rickets type 2; generalized arterial calcification of infancy; inorganic pyrophosphate.

Publication types

  • Observational Study
  • Research Support, Non-U.S. Gov't

MeSH terms

  • Adolescent
  • Alkaline Phosphatase / genetics
  • Alkaline Phosphatase / metabolism
  • Biomarkers / blood
  • Child
  • Child, Preschool
  • Enzyme Assays / methods
  • Enzyme Assays / standards
  • Familial Hypophosphatemic Rickets / blood
  • Familial Hypophosphatemic Rickets / diagnosis*
  • Familial Hypophosphatemic Rickets / genetics
  • Female
  • Humans
  • Hypophosphatasia / blood
  • Hypophosphatasia / diagnosis*
  • Hypophosphatasia / genetics
  • Infant
  • Infant, Newborn
  • Male
  • Multidrug Resistance-Associated Proteins / genetics
  • Multidrug Resistance-Associated Proteins / metabolism
  • Mutation
  • Phosphates / blood*
  • Phosphates / metabolism
  • Phosphoric Diester Hydrolases / genetics
  • Phosphoric Diester Hydrolases / metabolism
  • Pseudoxanthoma Elasticum / blood
  • Pseudoxanthoma Elasticum / diagnosis*
  • Pseudoxanthoma Elasticum / genetics
  • Pyrophosphatases / genetics
  • Pyrophosphatases / metabolism
  • Rare Diseases / blood
  • Rare Diseases / diagnosis*
  • Rare Diseases / genetics
  • Reference Values
  • Sulfate Adenylyltransferase / metabolism

Substances

  • ABCC6 protein, human
  • Biomarkers
  • Multidrug Resistance-Associated Proteins
  • Phosphates
  • Sulfate Adenylyltransferase
  • ALPL protein, human
  • Alkaline Phosphatase
  • Phosphoric Diester Hydrolases
  • ectonucleotide pyrophosphatase phosphodiesterase 1
  • Pyrophosphatases

Supplementary concepts

  • Hypophosphatemic Rickets, Autosomal Recessive, 2