Elastocaloric signature of nematic fluctuations

Proc Natl Acad Sci U S A. 2021 Sep 14;118(37):e2105911118. doi: 10.1073/pnas.2105911118.

Abstract

The elastocaloric effect (ECE) relates changes in entropy to changes in strain experienced by a material. As such, ECE measurements can provide valuable information about the entropy landscape proximate to strain-tuned phase transitions. For ordered states that break only point symmetries, bilinear coupling of the order parameter with strain implies that the ECE can also provide a window on fluctuations above the critical temperature and hence, in principle, can also provide a thermodynamic measure of the associated susceptibility. To demonstrate this, we use the ECE to sensitively reveal the presence of nematic fluctuations in the archetypal Fe-based superconductor Ba([Formula: see text])2[Formula: see text] By performing these measurements simultaneously with elastoresistivity in a multimodal fashion, we are able to make a direct and unambiguous comparison of these closely related thermodynamic and transport properties, both of which are sensitive to nematic fluctuations. As a result, we have uncovered an unanticipated doping dependence of the nemato-elastic coupling and of the magnitude of the scattering of low-energy quasi-particles by nematic fluctuations-while the former weakens, the latter increases dramatically with increasing doping.

Keywords: elastocaloric effect; iron pnictide superconductors; nematic fluctuations.

Publication types

  • Research Support, Non-U.S. Gov't
  • Research Support, U.S. Gov't, Non-P.H.S.