Induction of estrogen receptor β-mediated autophagy sensitizes breast cancer cells to TAD1822-7, a novel biphenyl urea taspine derivative

Mol Biol Rep. 2022 Feb;49(2):1223-1232. doi: 10.1007/s11033-021-06950-5. Epub 2021 Nov 18.

Abstract

Background: Female breast cancer has become the most commonly diagnosed cancer worldwide. As a tumor suppressor, estrogen receptor β (ERβ) can be potentially targeted for breast cancer therapy.

Methods and results: TAD1822-7 was evaluated for ERβ-mediated autophagy and cell death using cell proliferation assay, Annexin V/PI staining, immunofluorescence, western blotting, ERβ siRNA, ERβ plasmid transfection and hypoxia cell models. TAD1822-7 upregulated ERβ causing cell death and induced mitochondrial dysfunction and autophagy companied with mitochondrial located ERβ. Enhanced levels of microtubule associated protein1 light chain 3 (LC3)-II and p62/SQSTM1 (p62) indicated that TAD1822-7 blocked the late-stage autolysosome formation, leading to cell death. Mechanistically, TAD1822-7-induced cell death was mediated by phosphatidylinositol 3-kinase/protein kinase B (PI3K/AKT) signaling pathways. Moreover, TAD1822-7 modulated hypoxia inducible factor (HIF) functions and autophagy via the inhibition of HIF-1β in the context of hypoxia-induced autophagy. ERβ overexpression and ERβ agonist showed similar effects, whereas ERβ siRNA abrogated TAD1822-7-induced cell death, the inhibition of PI3K/AKT pathway and autophagy. The involvement of PI3K/AKT pathway and autophagy was also demonstrated in TAD1822-7-treated hypoxic breast cancer cells.

Conclusions: These findings provide new insight into the mechanism underlying the inhibitory effects of TAD1822-7 via ERβ-mediated pathways in breast cancer cells.

Keywords: Autophagy; Breast cancer; Cell death; Estrogen receptor β; Hypoxia; TAD1822-7.

MeSH terms

  • Alkaloids
  • Antineoplastic Agents / pharmacology
  • Apoptosis / drug effects
  • Autophagy / drug effects
  • Autophagy / physiology
  • Biphenyl Compounds
  • Breast Neoplasms / drug therapy*
  • Breast Neoplasms / metabolism
  • Cell Hypoxia / drug effects
  • Cell Line, Tumor
  • Cell Proliferation / drug effects
  • Estrogen Receptor beta / metabolism*
  • Estrogen Receptor beta / physiology
  • Female
  • Humans
  • Morpholines / metabolism
  • Morpholines / pharmacology*
  • Phenylurea Compounds / metabolism
  • Phenylurea Compounds / pharmacology*
  • Phosphatidylinositol 3-Kinases / metabolism
  • Proto-Oncogene Proteins c-akt / metabolism
  • Signal Transduction / drug effects
  • Urea

Substances

  • Alkaloids
  • Antineoplastic Agents
  • Biphenyl Compounds
  • Estrogen Receptor beta
  • Morpholines
  • Phenylurea Compounds
  • TAD1822-7
  • diphenyl
  • Urea
  • AKT1 protein, human
  • Proto-Oncogene Proteins c-akt
  • taspine