Anti-HIV Compounds from the Deep-Sea-Derived Fungus Chaetomium globosum

Chem Biodivers. 2022 Jan;19(1):e202100804. doi: 10.1002/cbdv.202100804. Epub 2021 Dec 16.

Abstract

Chemical investigation on the deep-sea-derived fungus Chaetomium globosum led to the isolation of nine compounds. By extensive analyses of the 1D and 2D NMR as well as HR-ESI-MS spectra, their structures were elucidated as xylariol A (1), 1,3-dihydro-4,5,6-trihydroxy-7-methylisobenzofuran (2), epicoccone B (3), epicoccolide B (4), chaetoglobosin G (5), chaetoglobosin Fex (6), cochliodone A (7), cochliodone B (8), and chaetoviridin A (9), assorting as four phenolics (1-4), two cytochalosans (5-6), and three azaplilones (7-9). Compounds 1-3 were firstly reported from C. globosum. Under the concentrations of 20 μg/mL, 1, 2, and 3 exhibited potent in vitro anti-HIV activity with the inhibition rates of 70 %, 75 %, and 88 %, respectively.

Keywords: Chaetomium globosum; anti-HIV; deep-sea; fungus; phenolics.

MeSH terms

  • Anti-HIV Agents / chemistry*
  • Anti-HIV Agents / isolation & purification
  • Anti-HIV Agents / pharmacology
  • Cell Line
  • Chaetomium / chemistry*
  • Chaetomium / metabolism
  • Genes, Reporter / drug effects
  • Humans
  • Magnetic Resonance Spectroscopy
  • Molecular Conformation
  • Phenols / chemistry
  • Phenols / isolation & purification
  • Phenols / pharmacology
  • Seawater / microbiology*
  • Spectrometry, Mass, Electrospray Ionization

Substances

  • Anti-HIV Agents
  • Phenols

Supplementary concepts

  • Chaetomium globosum