Cryo-EM structures of intermediates suggest an alternative catalytic reaction cycle for cytochrome c oxidase

Nat Commun. 2021 Nov 25;12(1):6903. doi: 10.1038/s41467-021-27174-y.

Abstract

Cytochrome c oxidases are among the most important and fundamental enzymes of life. Integrated into membranes they use four electrons from cytochrome c molecules to reduce molecular oxygen (dioxygen) to water. Their catalytic cycle has been considered to start with the oxidized form. Subsequent electron transfers lead to the E-state, the R-state (which binds oxygen), the P-state (with an already split dioxygen bond), the F-state and the O-state again. Here, we determined structures of up to 1.9 Å resolution of these intermediates by single particle cryo-EM. Our results suggest that in the O-state the active site contains a peroxide dianion and in the P-state possibly an intact dioxygen molecule, the F-state may contain a superoxide anion. Thus, the enzyme's catalytic cycle may have to be turned by 180 degrees.

Publication types

  • Research Support, Non-U.S. Gov't

MeSH terms

  • Catalysis*
  • Cryoelectron Microscopy*
  • Electron Transport Complex IV / chemistry*
  • Electron Transport Complex IV / metabolism*
  • Electrons
  • Escherichia coli
  • Membrane Proteins
  • Models, Molecular
  • Oxygen / metabolism
  • Paracoccus denitrificans
  • Peroxides / metabolism
  • Protons

Substances

  • Membrane Proteins
  • Peroxides
  • Protons
  • Electron Transport Complex IV
  • Oxygen