S-540956, a CpG Oligonucleotide Annealed to a Complementary Strand With an Amphiphilic Chain Unit, Acts as a Potent Cancer Vaccine Adjuvant by Targeting Draining Lymph Nodes

Front Immunol. 2021 Dec 23:12:803090. doi: 10.3389/fimmu.2021.803090. eCollection 2021.

Abstract

Robust induction of cancer-antigen-specific CD8+ T cells is essential for the success of cancer peptide vaccines, which are composed of a peptide derived from a cancer-specific antigen and an immune-potentiating adjuvant, such as a Toll-like receptor (TLR) agonist. Efficient delivery of a vaccine antigen and an adjuvant to antigen-presenting cells in the draining lymph nodes (LNs) holds key to maximize vaccine efficacy. Here, we developed S-540956, a novel TLR9-agonistic adjuvant consisting of B-type CpG ODN2006 (also known as CpG7909), annealed to its complementary sequence oligodeoxynucleotide (ODN) conjugated to a lipid; it could target both a cancer peptide antigen and a CpG-adjuvant in the draining LNs. S-540956 accumulation in the draining LNs and activation of plasmacytoid dendritic cells (pDCs) were significantly higher than that of ODN2006. Mechanistic analysis revealed that S-540956 enhanced the induction of MHC class I peptide-specific CD8+ T cell responses via TLR9 in a CD4+ T cell-independent manner. In mice, the therapeutic effect of S-540956-adjuvanted with a human papillomavirus (HPV)-E7 peptide vaccine against HPV-E7-expressing TC-1 tumors was significantly better than that of an ODN2006-adjuvanted vaccine. Our findings demonstrate a novel adjuvant discovery with the complementary strand conjugated to a lipid, which enabled draining LN targeting and increased ODN2006 accumulation in draining LNs, thereby enhancing the adjuvant effect. Our findings imply that S-540956 is a promising adjuvant for cancer peptide vaccines and has a high potential for applications in various vaccines, including recombinant protein vaccines.

Keywords: CpG oligonucleotide; adjuvant; cancer peptide vaccine; delivery system; draining lymph node.

Publication types

  • Research Support, Non-U.S. Gov't

MeSH terms

  • Adjuvants, Vaccine / chemistry
  • Adjuvants, Vaccine / therapeutic use*
  • Animals
  • CD8-Positive T-Lymphocytes / immunology*
  • Cancer Vaccines / immunology*
  • Cell Differentiation
  • DNA / chemistry
  • Dendritic Cells / immunology*
  • Female
  • Humans
  • Immunization
  • Lung Neoplasms / immunology*
  • Lymphocyte Activation
  • Mice
  • Mice, Inbred C57BL
  • Neoplasms, Experimental
  • Oligodeoxyribonucleotides / administration & dosage*
  • Oligodeoxyribonucleotides / chemistry
  • Papillomavirus E7 Proteins / immunology*
  • Sentinel Lymph Node / immunology*
  • Surface-Active Agents / chemistry
  • Toll-Like Receptor 9 / agonists
  • Toll-Like Receptor 9 / genetics
  • Toll-Like Receptor 9 / metabolism*
  • Vaccines, Subunit

Substances

  • Adjuvants, Vaccine
  • CPG-oligonucleotide
  • Cancer Vaccines
  • ODN2006
  • Oligodeoxyribonucleotides
  • Papillomavirus E7 Proteins
  • Surface-Active Agents
  • Toll-Like Receptor 9
  • Vaccines, Subunit
  • oncogene protein E7, Human papillomavirus type 16
  • DNA