Selective targeting of metastatic ovarian cancer using an engineered anthrax prodrug activated by membrane-anchored serine proteases

Proc Natl Acad Sci U S A. 2022 Jul 12;119(28):e2201423119. doi: 10.1073/pnas.2201423119. Epub 2022 Jul 8.

Abstract

Treatments for advanced and recurrent ovarian cancer remain a challenge due to a lack of potent, selective, and effective therapeutics. Here, we developed the basis for a transformative anticancer strategy based on anthrax toxin that has been engineered to be selectively activated by the catalytic power of zymogen-activating proteases on the surface of malignant tumor cells to induce cell death. Exposure to the engineered toxin is cytotoxic to ovarian tumor cell lines and ovarian tumor spheroids derived from patient ascites. Preclinical studies demonstrate that toxin treatment induces tumor regression in several in vivo ovarian cancer models, including patient-derived xenografts, without adverse side effects, supportive of progression toward clinical evaluation. These data lay the groundwork for developing therapeutics for treating women with late-stage and recurrent ovarian cancers, utilizing a mechanism distinct from current anticancer therapies.

Keywords: anthrax toxin; ascites; membrane-anchored serine proteases; metastatic ovarian cancer; prodrug.

Publication types

  • Research Support, N.I.H., Extramural
  • Research Support, Non-U.S. Gov't

MeSH terms

  • Antigens, Bacterial* / pharmacology
  • Antigens, Bacterial* / therapeutic use
  • Antineoplastic Agents* / pharmacology
  • Antineoplastic Agents* / therapeutic use
  • Bacterial Toxins* / pharmacology
  • Bacterial Toxins* / therapeutic use
  • Cell Line, Tumor
  • Enzyme Precursors / metabolism
  • Female
  • Humans
  • Neoplasm Recurrence, Local
  • Ovarian Neoplasms* / drug therapy
  • Ovarian Neoplasms* / pathology
  • Prodrugs* / pharmacology
  • Prodrugs* / therapeutic use
  • Serine Proteases* / metabolism
  • Spheroids, Cellular
  • Xenograft Model Antitumor Assays

Substances

  • Antigens, Bacterial
  • Antineoplastic Agents
  • Bacterial Toxins
  • Enzyme Precursors
  • Prodrugs
  • anthrax toxin
  • Serine Proteases