Economical Access to Diverse Enantiopure Tetrahydropyridines and Piperidines Enabled by Catalytic Borrowing Hydrogen

Angew Chem Int Ed Engl. 2023 Jan 9;62(2):e202212528. doi: 10.1002/anie.202212528. Epub 2022 Dec 7.

Abstract

We disclose herein a catalytic borrowing hydrogen method that enables an unprecedented, economical one-pot access to enantiopure tetrahydropyridines with minimal reagent use or waste formation. This method couples a few classes of readily available substrates with commercially available 1,3-amino alcohols, and delivers the valuable tetrahydropyridines of different substitution patterns free of N-protection. Such transformations are highly challenging to achieve, as multiple redox steps need to be realized in a cascade and numerous side reactions including a facile aromatization have to be overcome. Highly diastereoselective functionalizations of tetrahydropyridines also result in a general access to enantiopure di- and tri-substituted piperidines, which ranks the topmost frequent N-heterocycle in commercial drugs.

Keywords: Borrowing Hydrogen; Heterocycle; Piperidine; Redox Economy; Tetrahydropyridine.

Publication types

  • Research Support, Non-U.S. Gov't

MeSH terms

  • Hydrogen
  • Molecular Structure
  • Piperidines*
  • Pyrrolidines*
  • Stereoisomerism

Substances

  • Piperidines
  • Pyrrolidines
  • Hydrogen