Highly selective pressure-dependent (transfer) hydrogenative depolymerization of polybutylene succinate

Chem Commun (Camb). 2024 Jan 16;60(6):702-705. doi: 10.1039/d3cc05239g.

Abstract

Ru-MACHO®-BH is an effective catalyst for controlled depolymerization of polybutylene succinate. Under low pressure hydrogen the catalyst produces gamma-butyrolactone via a novel transfer hydrogenation wherein dehydrogenation and hydrogenation deconstruct the polymer chain. Simply increasing the hydrogen pressure selectively generates 1,4-butanediol.