Biosensor Strip for Rapid On-site Assessment of Levodopa Pharmacokinetics along with Motor Performance in Parkinson's Disease

Angew Chem Int Ed Engl. 2024 Jul 1;63(27):e202403583. doi: 10.1002/anie.202403583. Epub 2024 May 28.

Abstract

While levodopa (L-Dopa) is the primary treatment for alleviating Parkinson's disease (PD), its efficacy is hindered by challenges such as a short half-life and inconsistent plasma levels. As PD progresses, the rising need for increased and more frequent L-Dopa doses coupled with symptom fluctuations and dyskinesias underscores the urgency for improved comprehension of the interplay between L-Dopa levels and PD motor symptoms. Addressing this critical need, we present a decentralized testing method using a disposable biosensor strip and a universal slope (U-slope) calibration-free approach. This enables reliable, rapid, simple, and cost-effective decentralized L-Dopa measurements from capillary blood. A pilot study with PD persons demonstrates the ability to monitor real-time L-Dopa pharmacokinetics from fingerstick blood after oral L-Dopa-Carbidopa (C-Dopa) tablet administration. Correlating capillary blood L-Dopa levels with PD motor scores revealed a well-defined inverse correlation with temporal motor fluctuations. We compared the resulting dynamic capillary blood L-Dopa levels with plasma L-Dopa levels using the traditional but clinically impractical high-performance liquid chromatography technique. By providing timely feedback on a proper L-Dopa dosing regimen in a decentralized and rapid fashion, this new biosensing platform will facilitate tailored optimal L-Dopa dosing, towards improving symptom management and enhancing health-related quality of life.

Keywords: biosensor; levodopameter; levodopastrip; near-realtime TDM; parkinsons management.

Publication types

  • Research Support, N.I.H., Extramural

MeSH terms

  • Antiparkinson Agents / administration & dosage
  • Antiparkinson Agents / blood
  • Antiparkinson Agents / pharmacokinetics
  • Antiparkinson Agents / therapeutic use
  • Biosensing Techniques*
  • Carbidopa / administration & dosage
  • Carbidopa / pharmacokinetics
  • Carbidopa / therapeutic use
  • Humans
  • Levodopa* / blood
  • Levodopa* / chemistry
  • Levodopa* / pharmacokinetics
  • Levodopa* / therapeutic use
  • Male
  • Parkinson Disease* / drug therapy
  • Pilot Projects

Substances

  • Levodopa
  • Antiparkinson Agents
  • Carbidopa