Enantioselective α-heterofunctionalization reactions of catalytically generated C1-Lewis base enolates

Tetrahedron Chem. 2024 Mar:9:100063. doi: 10.1016/j.tchem.2024.100063.

Abstract

Chiral Lewis base (LB) organocatalysis has emerged as a powerful covalent catalysis concept which allows for highly selective asymmetric C-C and C-heteroatom bond formations. Considering significant recent progress in the development of strategies to access α-heterofunctionalized carboxylic acid derivatives under chiral LB catalysis, we wish to summarize the most significant concepts and advances in this field within this mini review now.

Keywords: Carboxylic acid derivatives; Covalent catalysis; Heterofunctionalizations; Lewis bases; Organocatalysis.