6-shogaol against 3-Nitropropionic acid-induced Huntington's disease in rodents: Based on molecular docking/targeting pro-inflammatory cytokines/NF-κB-BDNF-Nrf2 pathway

PLoS One. 2024 Jul 15;19(7):e0305358. doi: 10.1371/journal.pone.0305358. eCollection 2024.

Abstract

Background: Huntington's disease (HD) is an extremely harmful autosomal inherited neurodegenerative disease. Motor dysfunction, mental disorder, and cognitive deficits are the characteristic features of this disease. The current study examined whether 6-shogaol has a protective effect against 3-Nitropropionic Acid (3-NPA)-induced HD in rats.

Methods: A total of thirty male Wistar rats received 6-shogaol (10 and 20 mg/kg, per oral) an hour before injection of 3-NPA (10 mg/kg i.p.) for 15 days. Behavioral tests were performed, including narrow beam walk, rotarod test, and grip strength test. Biochemical tests promoting oxidative stress were evaluated [superoxide dismutase (SOD), reduced glutathione (GSH), catalase (CAT) and malondialdehyde (MDA)], including changes to neurotransmitters serotonin (5-HT), dopamine (DA), norepinephrine (NE), homovanillic acid (HVA), (3,4-dihydroxyphenylacetic acid (DOPAC), γ-aminobutyric acid (GABA), and 5-hydroxy indole acetic acid (5-HIAA), nuclear factor kappa-B (NF-κB), tumor necrosis factor-α (TNF-α), interleukins-1β (IL-1β), IL-6, brain-derived neurotrophic factor (BDNF), and nuclear factor erythroid 2-related factor 2 (Nrf2). The 6-shogaol was docked to the active site of TNF-α (2AZ5), NF-κB (1SVC), BDNF) [1B8M], and Nrf2 [5FZN] proteins using AutoDock tools.

Results: The 6-shogaol group significantly improved behavioral activity over the 3-NPA-injected control rats. Moreover, 3-NPA-induced significantly altered neurotransmitters, biochemical and neuroinflammatory indices, which could efficiently be reversed by 6-shogaol. The 6-shogaol showed favorable negative binding energies at -9.271 (BDNF) kcal/mol.

Conclusions: The present investigation demonstrated the neuroprotective effects of 6-shogaol in an experimental animal paradigm against 3-NPA-induced HD in rats. The suggested mechanism is supported by immunohistochemical analysis and western blots, although more research is necessary for definite confirmation.

MeSH terms

  • Animals
  • Behavior, Animal / drug effects
  • Brain-Derived Neurotrophic Factor* / metabolism
  • Catechols* / chemistry
  • Catechols* / pharmacology
  • Cytokines* / metabolism
  • Huntington Disease* / chemically induced
  • Huntington Disease* / drug therapy
  • Huntington Disease* / metabolism
  • Male
  • Molecular Docking Simulation*
  • NF-E2-Related Factor 2* / metabolism
  • NF-kappa B* / metabolism
  • Neuroprotective Agents / pharmacology
  • Nitro Compounds*
  • Oxidative Stress / drug effects
  • Propionates* / pharmacology
  • Rats
  • Rats, Wistar*
  • Signal Transduction / drug effects

Substances

  • 3-nitropropionic acid
  • Propionates
  • Brain-Derived Neurotrophic Factor
  • Nitro Compounds
  • NF-kappa B
  • NF-E2-Related Factor 2
  • Catechols
  • Cytokines
  • shogaol
  • Nfe2l2 protein, rat
  • Bdnf protein, rat
  • Neuroprotective Agents

Grants and funding

This research work was funded by Researchers Supporting Project number (RSPD2024R552), King Saud University, Riyadh, Saudi Arabia.