Combination non-targeted and sGRP78-targeted nanoparticle drug delivery outperforms either component to treat metastatic ovarian cancer

J Control Release. 2024 Nov:375:438-453. doi: 10.1016/j.jconrel.2024.09.014. Epub 2024 Sep 19.

Abstract

Metastatic ovarian cancer (MOC) is highly deadly, due in part to the limited efficacy of standard-of-care chemotherapies to metastatic tumors and non-adherent cancer cells. Here, we demonstrated the effectiveness of a combination therapy of GRP78-targeted (TNPGRP78pep) and non-targeted (NP) nanoparticles to deliver a novel DM1-prodrug to MOC in a syngeneic mouse model. Cell surface-GRP78 is overexpressed in MOC, making GRP78 an optimal target for selective delivery of nanoparticles to MOC. The NP + TNPGRP78pep combination treatment reduced tumor burden by 15-fold, compared to untreated control. Increased T cell and macrophage levels in treated groups also suggested antitumor immune system involvement. The NP and TNPGRP78pep components functioned synergistically through two proposed mechanisms of action. The TNPGRP78pep targeted non-adherent cancer cells in the peritoneal cavity, preventing the formation of new solid tumors, while the NP passively targeted existing solid tumor sites, providing a sustained release of the drug to the tumor microenvironment.

Keywords: Antitumor immune response; Lipid nanoparticle; Metastasis; Ovarian cancer; Targeted drug delivery; women's health.

MeSH terms

  • Animals
  • Antineoplastic Agents / administration & dosage
  • Antineoplastic Agents / pharmacokinetics
  • Antineoplastic Agents / therapeutic use
  • Cell Line, Tumor
  • Endoplasmic Reticulum Chaperone BiP*
  • Female
  • Heat-Shock Proteins*
  • Humans
  • Maytansine / administration & dosage
  • Maytansine / analogs & derivatives
  • Maytansine / pharmacokinetics
  • Maytansine / therapeutic use
  • Mice
  • Mice, Inbred C57BL
  • Nanoparticle Drug Delivery System
  • Nanoparticles / administration & dosage
  • Ovarian Neoplasms* / drug therapy
  • Ovarian Neoplasms* / pathology

Substances

  • Endoplasmic Reticulum Chaperone BiP
  • Hspa5 protein, mouse
  • HSPA5 protein, human
  • Heat-Shock Proteins
  • Maytansine
  • Antineoplastic Agents
  • Nanoparticle Drug Delivery System