Electrochemical Growth of Copper Crystals on SPCE for Electrocatalysis Nitrate Reduction

Nanomaterials (Basel). 2024 Oct 24;14(21):1704. doi: 10.3390/nano14211704.

Abstract

Copper is efficient, has a high conductivity (5.8 × 107 S/m), and is cost-effective. The use of copper-based catalysts is promising for the electrocatalytic reduction of nitrates. This work aims to grow and characterize copper micro-crystals on Screen-Printed Electrodes (SPEs) for NO3- reduction in water. Copper micro-crystals were grown by cyclic voltammetry. Different cycles (2, 5, 7, 10, 12, 15) of copper electrodeposition were investigated (potential ranges from -1.0 V to 0.0 V, scan rate of 0.1 V s-1). Electrodeposition generated different morphologies of copper crystals on the electrodes, as a function of the number of cycles, with various performances. The presence of numerous edges and defects in the copper micro-crystal structures creates highly reactive active sites, thus favoring nitrate reduction. The manufactured material can be successfully employed for environmental applications.

Keywords: copper micro-flowers; cyclic voltammetry; electrochemical deposition; nitrate reduction.