Stretchable and High-Performance Fibrous Sensors Based on Ionic Capacitive Sensing for Wearable Healthcare Monitoring

Electronic textiles with remarkable breathability, lightweight, and comfort hold great potential in wearable technologies and smart human-machine interfaces. Ionic capacitive sensors, leveraging the advantages of the electric double layer, offer higher sensitivity compared to traditional capacitive sensors. Current research on wearable ion-capacitive sensors has focused mainly on two-dimensional (2D) or three-dimensional (3D) device architectures, which show substantial challenges for direct integration with textiles and compromise their wearing experience on conformability and permeability. One-dimensional (1D) stretchable fiber materials serve as vital components in constructing electronic textiles, allowing for rich structural design, patterning, and device integration through mature textile techniques. Here, a stretchable functional fiber with robust mechanical and electrical performances is fabricated based on semi-solid metal and ionic polymer, which provided a high stretchability and good electrical conductivity, enabling seamless integration with textiles. Consequently, high-performance stretchable fiber sensors are developed through different device architecture designs, including pressure sensors with high sensitivity (7.21 kPa^-1), fast response (60 ms/30 ms), and excellent stability, as well as strain sensors with high sensitivity (GF = 1.05), wide detection range (0-300% strain), and excellent sensing stability under dynamic deformations.