Three New Dipeptide and Two New Polyketide Derivatives from the Mangrove-Derived Fungus Talaromyces sp.: Antioxidant Activity of Two Isolated Substances

Mar Drugs. 2024 Dec 14;22(12):559. doi: 10.3390/md22120559.

Abstract

Five new metabolites, including three cyclic dipeptide derivatives (1-3) and two new polyketides (10-11), together with nine known ones (4-9 and 12-15), were isolated from the mangrove-sediments-derived fungus Talaromyces sp. SCSIO 41431. Their structures were determined using detailed NMR, MS spectroscopic analyses, and quantum chemical calculations. X-ray single-crystal diffraction analysis of 1 was described. Compounds 13-15 demonstrated activity against Staphylococcus aureus, with MIC values ranging from 25 to 50 µg/mL. Compound 9 showed activity against Escherichia coli, Streptococcus suis, and Erysipelothrix rhusiopathiae, with an MIC value of 100 µg/mL. In addition, compounds 1 and 12 showed DPPH radical scavenging activity, with the EC50 of 27.62 and 29.34 µg/mL, compared to the positive control (ascorbic acid, EC50, 12.74 µg/mL).

Keywords: DPPH; Talaromyces sp.; dipeptide; mangrove-derived fungus; polyketide.

MeSH terms

  • Anti-Bacterial Agents / chemistry
  • Anti-Bacterial Agents / isolation & purification
  • Anti-Bacterial Agents / pharmacology
  • Antioxidants* / chemistry
  • Antioxidants* / isolation & purification
  • Antioxidants* / pharmacology
  • Crystallography, X-Ray
  • Dipeptides* / chemistry
  • Dipeptides* / isolation & purification
  • Dipeptides* / pharmacology
  • Microbial Sensitivity Tests*
  • Molecular Structure
  • Polyketides* / chemistry
  • Polyketides* / isolation & purification
  • Polyketides* / pharmacology
  • Staphylococcus aureus / drug effects
  • Talaromyces* / chemistry

Substances

  • Polyketides
  • Antioxidants
  • Dipeptides
  • Anti-Bacterial Agents