Moroccan natural products for multitarget-based treatment of Alzheimer's disease: A computational study

PLoS One. 2025 Jan 16;20(1):e0313411. doi: 10.1371/journal.pone.0313411. eCollection 2025.

Abstract

Alzheimer's disease is a neurodegenerative disorder that impairs neurocognitive functions. Acetylcholinesterase, Butyrylcholinesterase, Monoamine Oxidase B, Beta-Secretase, and Glycogen Synthase Kinase Beta play central roles in its pathogenesis. Current medications primarily inhibit AChE but fail to halt or reverse disease progression due to the multifactorial nature of Alzheimer's. This underscores the necessity of developing multi-target ligands for effective treatment. This study investigates the potential of phytochemical compounds from Moroccan medicinal plants as multi-target agents against Alzheimer's disease, employing computational approaches. A virtual screening of 386 phytochemical compounds, followed by an assessment of pharmacokinetic properties and ADMET profiles, led to the identification of two promising compounds, naringenin (C23) and hesperetin (C24), derived from Anabasis aretioides. These compounds exhibit favourable pharmacokinetic profiles and strong binding affinities for the five key targets associated with the disease. Density functional theory, molecular dynamics simulations, and MM-GBSA calculations further confirmed their structural stability, with a slight preference for C24, exhibiting superior intermolecular interactions and overall stability. These findings provide a strong basis for further experimental research, including in vitro and in vivo studies, to substantiate their potential efficacy in Alzheimer's disease.

MeSH terms

  • Acetylcholinesterase / chemistry
  • Acetylcholinesterase / metabolism
  • Alzheimer Disease* / drug therapy
  • Biological Products / chemistry
  • Biological Products / pharmacology
  • Biological Products / therapeutic use
  • Flavanones / chemistry
  • Flavanones / pharmacology
  • Flavanones / therapeutic use
  • Hesperidin* / chemistry
  • Hesperidin* / pharmacology
  • Hesperidin* / therapeutic use
  • Humans
  • Molecular Docking Simulation
  • Molecular Dynamics Simulation
  • Morocco
  • Plants, Medicinal / chemistry

Substances

  • Hesperidin
  • naringenin
  • Biological Products
  • hesperetin
  • Flavanones
  • Acetylcholinesterase