Capillary gas chromatographic method for the analysis of lignans in human urine

Clin Chim Acta. 1982 Jun 3;121(3):361-71. doi: 10.1016/0009-8981(82)90245-5.

Abstract

We describe a capillary column gas chromatographic (GC) method for the analysis of lignans in urine. Lignans are excreted as mono-glucuronides which are first extracted on a small reversed-phase cartridge of octadecylsilane bonded silica (Sep-Pak C18) and thereafter isolated by anion exchange chromatography on DEAE-Sephadex A-25, prepared in the acetate form. Lignan mono-glucuronides are enzymatically hydrolysed and re-extracted on a Sep-Pak C18 cartridge. Quantification is carried out by capillary column GC of the trimethylsilyl ether derivatives. The specificity of the method was checked by GC/MS and the intra-assay coefficient of variation (CV) for the two lignans, enterolactone (trans-2,3-bis(3-hydroxybenzyl)butyrolactone) and enterodiol (2.3-bis(3-hydroxybenzyl)butane-1,4-diol) varied between 5 and 8%. Some values for the excretion of these lignans by normal men and women are presented.

Publication types

  • Comparative Study
  • Research Support, Non-U.S. Gov't
  • Research Support, U.S. Gov't, P.H.S.

MeSH terms

  • 4-Butyrolactone / analogs & derivatives
  • 4-Butyrolactone / urine
  • Adult
  • Butylene Glycols / urine
  • Chromatography, Gas / methods*
  • Chromatography, Ion Exchange
  • Female
  • Gas Chromatography-Mass Spectrometry
  • Glucuronates / urine
  • Humans
  • Lignans
  • Male
  • Middle Aged
  • Plant Extracts / urine*

Substances

  • Butylene Glycols
  • Glucuronates
  • Lignans
  • Plant Extracts
  • 2,3-bis(3'-hydroxybenzyl)butane-1,4-diol
  • 4-Butyrolactone
  • 2,3-bis(3'-hydroxybenzyl)butyrolactone