Characterization of the arachidonate and ATP binding sites of human 5-lipoxygenase using photoaffinity labeling and enzyme immobilization

Biochemistry. 1995 Oct 17;34(41):13603-11. doi: 10.1021/bi00041a040.

Abstract

The arachidonic acid and the ATP binding sites of human 5-lipoxygenase were characterized using photoaffinity labeling and immobilization of the enzyme on ATP-agarose. Photoaffinity labeling of the active site of 5-lipoxygenase was achieved with a novel thiopyranoindole inhibitor containing a 4-azido-3-iodobenzenesulfonyl moiety (L-708,714). This probe was found to inhibit the activity of 5-lipoxygenase (IC50 = 0.3 microM) and to covalently label the enzyme after UV light irradiation. The labeling was inhibited by arachidonic acid, N-hydroxyurea, and dihydrobenzofuranol inhibitors which have been shown to reduce the non-heme iron center of 5-lipoxygenase. Photoaffinity labeling of 5-lipoxygenase by L-708,714 was dependent on the presence of both Ca2+ ions and phospholipids and was independent of ATP. It occurred at similar levels using native (Fe2+), oxidized (Fe3+), or H2O2-inactivated enzyme, but was abolished by heat inactivation of the enzyme. Competition of the labeling by various thiopyranoindoles and other inhibitors such as L-697,198,ZD-2138, and zileuton was found to be related to their inhibitory potency. Immobilized 5-lipoxygenase on ATP-agarose was found to be selectively eluted by adenine nucleotides (ATP > ADP > AMP) but not by solutions containing high salt concentrations, mild detergents, arachidonic acid, or inhibitors. 5-Lipoxygenase inhibitors were selectively retained on the immobilized enzyme and eluted by buffer containing arachidonic acid.(ABSTRACT TRUNCATED AT 250 WORDS)

Publication types

  • Comparative Study

MeSH terms

  • Adenine Nucleotides / metabolism
  • Adenine Nucleotides / pharmacology
  • Adenosine Triphosphate / metabolism*
  • Affinity Labels
  • Animals
  • Arachidonate 5-Lipoxygenase / chemistry*
  • Arachidonate 5-Lipoxygenase / metabolism*
  • Arachidonate 5-Lipoxygenase / radiation effects
  • Arachidonic Acid / metabolism*
  • Arachidonic Acid / pharmacology
  • Binding Sites
  • Binding, Competitive
  • Calcium / pharmacology
  • Enzymes, Immobilized / chemistry*
  • Enzymes, Immobilized / metabolism*
  • Humans
  • Hydroxyurea / pharmacology
  • Indoles / chemical synthesis
  • Indoles / metabolism
  • Indoles / pharmacology*
  • Indomethacin / pharmacology
  • Iodobenzenes / metabolism
  • Iodobenzenes / pharmacology
  • Kinetics
  • Lipoxygenase Inhibitors / chemical synthesis
  • Lipoxygenase Inhibitors / pharmacology*
  • Phospholipids / pharmacology
  • Recombinant Proteins / chemistry
  • Recombinant Proteins / isolation & purification
  • Recombinant Proteins / metabolism
  • Sepharose / analogs & derivatives
  • Spodoptera
  • Structure-Activity Relationship
  • Transfection
  • Ultraviolet Rays

Substances

  • ATP-sepharose
  • Adenine Nucleotides
  • Affinity Labels
  • Enzymes, Immobilized
  • Indoles
  • Iodobenzenes
  • L 708714
  • Lipoxygenase Inhibitors
  • Phospholipids
  • Recombinant Proteins
  • Arachidonic Acid
  • Adenosine Triphosphate
  • Sepharose
  • Arachidonate 5-Lipoxygenase
  • Calcium
  • Hydroxyurea
  • Indomethacin