Enzymatic reduction of xenobiotic alpha,beta-unsaturated ketones: formation of allyl alcohol metabolites from shogaol and dehydroparadol

Res Commun Chem Pathol Pharmacol. 1994 Apr;84(1):53-61.

Abstract

A novel reductive metabolism of shogaol [1-(4'-hydroxy-3'-methoxyphenyl)-deca-4-ene-3-one], a major pungent and pharmacologically active principle of ginger, was investigated in rat liver in vitro. The ethyl acetate extractable metabolites formed by incubation of this alpha,beta-unsaturated ketone with rat liver 12,000 x g supernatant fortified with NADPH-generating system were analyzed by high performance chromatography and gas chromatography/mass spectrometry. In addition to the saturated ketone and reduced alcohol metabolites, an allyl alcohol, 1-(4'-hydroxy-3'-methoxyphenyl)-deca-4-ene-3-ol, was identified as a new metabolite of shogaol. Likewise, dehydroparadol [1-(4'-hydroxy-3'-methoxyphenyl)-deca-1-ene-3-one], a non-pungent analog of shogaol, was also reduced to the corresponding allyl alcohol by the postmitochondrial fraction of rat kidney in the presence of NADPH-generating system.

Publication types

  • Research Support, Non-U.S. Gov't

MeSH terms

  • 1-Propanol / metabolism
  • Allyl Compounds / metabolism
  • Animals
  • Catechols / chemical synthesis
  • Catechols / metabolism*
  • Chromatography, High Pressure Liquid
  • Gas Chromatography-Mass Spectrometry
  • Guaiacol / analogs & derivatives*
  • Guaiacol / metabolism
  • Kidney / enzymology
  • Kidney / metabolism*
  • Liver / enzymology
  • Liver / metabolism*
  • Male
  • Mutagens / chemical synthesis
  • Mutagens / metabolism*
  • Oxidation-Reduction
  • Plant Extracts / metabolism*
  • Propanols
  • Rats
  • Rats, Sprague-Dawley

Substances

  • Allyl Compounds
  • Catechols
  • Mutagens
  • Plant Extracts
  • Propanols
  • allyl alcohol
  • dehydroparadol
  • Guaiacol
  • shogaol
  • 1-Propanol