Enzymic reduction of [6]-gingerol, a major pungent principle of ginger, in the cell-free preparation of rat liver

Life Sci. 1994;54(19):PL321-6. doi: 10.1016/0024-3205(94)00602-4.

Abstract

A reductive metabolism of S-(+)-[6]-gingerol [1-(4'-hydroxy-3'-methoxyphenyl)-5-hydroxydecan-3-one], the major pungent principle of ginger, was investigated in vitro with phenobarbital-induced rat liver 10,000 x g supernatant containing the NADPH-generating system. The ethyl acetate-extractable products were isolated and two metabolites were identified as diastereomers of [6]-gingerdiol by gas chromatography/mass spectrometry. The ratio of two isomers formed in the above reaction was about 1:5, suggesting the stereospecific reduction of S-(+)-[6]-gingerol by carbonyl reductase activity present in the postmitochondrial supernatant fraction of rat liver. The enzymic reduction of S-(+)-[6]-gingerol thus introduces the second asymmetric carbon center in the molecule with concomitant production of S,S- and R,S-isomers of [6]-gingerdiol in different proportions. This stereospecific reduction of [6]-gingerol may be relevant to the clinical use of the compound.

Publication types

  • Research Support, Non-U.S. Gov't

MeSH terms

  • Animals
  • Catechols
  • Cell-Free System
  • Chromatography, Thin Layer
  • Fatty Alcohols / chemistry
  • Fatty Alcohols / metabolism*
  • Gas Chromatography-Mass Spectrometry
  • Liver / drug effects
  • Liver / metabolism*
  • Male
  • Molecular Structure
  • Oxidation-Reduction
  • Phenobarbital / pharmacology
  • Plants, Medicinal
  • Rats
  • Rats, Sprague-Dawley
  • Spices

Substances

  • Catechols
  • Fatty Alcohols
  • gingerol
  • Phenobarbital