Antipicornavirus activity of tetrazole analogues related to disoxaril

J Med Chem. 1993 Oct 29;36(22):3240-50. doi: 10.1021/jm00074a004.

Abstract

A series of tetrazole analogues of Win 54954, a broad-spectrum antipicornavirus compound, has been synthesized to address the acid lability of the oxazoline ring of this series of compounds. The results of X-ray crystallography studies of several members of the oxazoline series bound to human rhinovirus type 1A and 14 have been used to design compounds in the tetrazole series with a broad spectrum of activity. Compound 16b, which has a three-carbon linkage between the isoxazole and phenyl rings and a propyl chain extending from the isoxazole ring, exhibiting an MIC80 for 15 rhinovirus serotypes of 0.20 microM as compared to 0.40 microM for Win 54954. X-ray studies of 16b bound to human rhinovirus-14 show that the propyl side chain extends into a pore in the binding site with the possibility of hydrophobic interactions with a pocket formed by Leu106 and a portion of Ser107.

Publication types

  • Comparative Study

MeSH terms

  • Amino Acid Sequence
  • Antiviral Agents / chemical synthesis*
  • Antiviral Agents / pharmacology*
  • Binding Sites
  • Humans
  • Isoxazoles / chemical synthesis*
  • Isoxazoles / chemistry
  • Isoxazoles / pharmacology*
  • Microbial Sensitivity Tests
  • Molecular Sequence Data
  • Picornaviridae / drug effects*
  • Rhinovirus / drug effects
  • Structure-Activity Relationship
  • Tetrazoles / chemical synthesis*
  • Tetrazoles / pharmacology*

Substances

  • Antiviral Agents
  • Isoxazoles
  • Tetrazoles
  • Win 54954
  • disoxaril