Observation of "hook effects" in the inhibition and dose-response curves of biotin assays based on the interaction of biotinylated glucose oxidase with (strept)avidin

Anal Chem. 1993 Feb 15;65(4):457-60. doi: 10.1021/ac00052a024.

Abstract

The inhibition of highly biotinylated enzymes by avidin and streptavidin has been used in the development of homogeneous assays for biotin and other analytes. Usually, this inhibition occurs in a similar fashion for both avidin and streptavidin. Specifically, the curves that relate the inhibition of the enzymatic activity with the concentration of avidin or streptavidin have a sigmoidal shape; I.e., the inhibition of the enzyme-biotin conjugates increases gradually with increasing amounts of avidin or streptavidin and arrives at a plateau at high binding protein concentrations. However, when these two biotin-specific binding proteins interact with biotinylated glucose oxidase a significant difference in their inhibitory action is observed. In particular, the inhibition curves have a sigmoidal shape for streptavidin, while those for avidin exhibit a maximum ("hook") at low avidin concentrations. This difference in the reactivity of the two proteins with biotinylated enzymes influences both the shape of the dose-response curve and the detection limits of homogeneous enzyme-linked competitive binding assays for biotin.

Publication types

  • Research Support, U.S. Gov't, P.H.S.

MeSH terms

  • Avidin / metabolism*
  • Bacterial Proteins / metabolism*
  • Binding, Competitive
  • Biotin / analysis*
  • Carrier Proteins
  • Dose-Response Relationship, Drug
  • Glucose Oxidase / metabolism*
  • Streptavidin

Substances

  • Bacterial Proteins
  • Carrier Proteins
  • Avidin
  • Biotin
  • Streptavidin
  • Glucose Oxidase