Human isopentenyl diphosphate: dimethylallyl diphosphate isomerase: overproduction, purification, and characterization

Arch Biochem Biophys. 1996 Aug 1;332(1):30-4. doi: 10.1006/abbi.1996.0312.

Abstract

Isopentenyl diphosphate (IPP):dimethylallyl diphosphate isomerase catalyzes an essential activation step in the isoprenoid biosynthetic pathway. A human cDNA sequence [J. Xuan, J. Kowalski, A.F. Chambers, and D.T. Denhardt (1994) Genomics 20, 129-131] containing a 684-base-pair open reading frame was recently reported that encoded a protein with a significant degree of similarity to two fungal IPP isomerases [F.M. Hahn and C.D. Poulter (1995) J. Biol. Chem. 270, 11298-11303]. The human cDNA sequence was cloned into expression plasmid pFMH12. The encoded protein was overproduced in Escherichia coli and purified to > 90% homogeneity in two steps by ion-exchange and hydrophobic interaction chromatography. The recombinant protein catalyzed the isomerization of IPP to dimethylallyl diphosphate and was maximally active at pH 7.0 in the presence of Mg2+. The Michaelis constant for IPP was 33 microM, similar to the value of 43 microM reported for yeast IPP isomerase; Vmax = 4.1 mumol min-1 mg-1 for recombinant human IPP isomerase, approximately fivefold less than reported for the yeast enzyme [I.P. Street and C.D. Poulter (1990) Biochemistry 29, 7531-7538].

Publication types

  • Research Support, Non-U.S. Gov't
  • Research Support, U.S. Gov't, P.H.S.

MeSH terms

  • Amino Acid Sequence
  • Base Sequence
  • Carbon-Carbon Double Bond Isomerases*
  • Cloning, Molecular
  • DNA Primers / genetics
  • DNA, Complementary / genetics
  • Escherichia coli / genetics
  • Hemiterpenes
  • Humans
  • Hydrogen-Ion Concentration
  • Isomerases / biosynthesis*
  • Isomerases / genetics
  • Isomerases / isolation & purification*
  • Kinetics
  • Molecular Sequence Data
  • Open Reading Frames
  • Recombinant Proteins / biosynthesis
  • Recombinant Proteins / genetics
  • Recombinant Proteins / isolation & purification
  • Sequence Homology, Amino Acid

Substances

  • DNA Primers
  • DNA, Complementary
  • Hemiterpenes
  • Recombinant Proteins
  • Isomerases
  • Carbon-Carbon Double Bond Isomerases
  • isopentenyldiphosphate delta-isomerase