Use of LC-MS/MS to cross-validate a radioimmunoassay for the fibrinogen receptor antagonist, Aggrastat (tirofiban hydrochloride) in human plasma

J Pharm Biomed Anal. 1997 Feb;15(5):561-9. doi: 10.1016/s0731-7085(96)01848-1.

Abstract

A method based on LC-MS/MS was developed for the determination of the fibrinogen-receptor antagonist Aggrastat in human plasma. The drug is isolated from plasma by liquid extraction and converted into its N-trifluoroacetyl derivative prior to analysis by HPLC with atmospheric pressure negative chemical ionization MS/MS detection. A structural analog is used as the internal standard and the lower quantifiable limit of the assay is 0.4 ng ml-1 with a relative standard deviation of 7%. This assay was used to cross-validate the existing immunoassay by analysis of plasma from patients receiving the drug. The specificity of the immunoassay was thereby confirmed.

MeSH terms

  • Calibration
  • Chromatography, Liquid / methods
  • Fibrinolytic Agents / blood*
  • Humans
  • Mass Spectrometry / methods
  • Platelet Aggregation Inhibitors / blood*
  • Platelet Glycoprotein GPIIb-IIIa Complex / antagonists & inhibitors*
  • Radioimmunoassay
  • Reproducibility of Results
  • Sensitivity and Specificity
  • Tirofiban
  • Tyrosine / analogs & derivatives*
  • Tyrosine / blood

Substances

  • Fibrinolytic Agents
  • Platelet Aggregation Inhibitors
  • Platelet Glycoprotein GPIIb-IIIa Complex
  • Tyrosine
  • Tirofiban