Improved resolution in the detection of oligonucleotides up to 60-mers in matrix-assisted laser desorption/ionization time-of-flight mass spectrometry using pulsed-delayed extraction with a simple high voltage transistor switch

Rapid Commun Mass Spectrom. 1997;11(9):987-92. doi: 10.1002/(SICI)1097-0231(19970615)11:9<987::AID-RCM949>3.0.CO;2-J.

Abstract

Pulsed-delayed extraction using a simple high voltage transistor switch together with various sample purification approaches were used to enhance the resolution in matrix-assisted laser desorption/ionization time-of-flight mass spectrometry (MALDI-TOFMS) of oligonucleotides up to 60 bases long. This switch can provide a 0-3 kV voltage pulse with a 75 ns fall time. A resolution of 500-900 was typically observed for samples from 5-mers to 60-mers using pulsed-delayed extraction (PDE) with the switch described herein. The resolution deteriorated to < 100 for oligonucleotides of > or = 65-mers. With the TOF acceleration region configuration used in this work, the resolution was found not to vary significantly over a delay range of 2-5 mus. As the DNA size increased to over 35-mer, HPLC purification was required to retain the enhancement in resolution provided by PDE MALDI-MS.

Publication types

  • Research Support, U.S. Gov't, P.H.S.

MeSH terms

  • Chromatography, High Pressure Liquid
  • DNA / analysis
  • Oligonucleotides / analysis*
  • Oligonucleotides / isolation & purification
  • Spectrometry, Mass, Matrix-Assisted Laser Desorption-Ionization / instrumentation*
  • Transistors, Electronic

Substances

  • Oligonucleotides
  • DNA