The structures of polysaccharides and glycolipids of Aspergillus fumigatus grown in the presence of human serum

Mycopathologia. 1997;137(1):17-25. doi: 10.1023/a:1006862420963.

Abstract

A study was made of polysaccharides and glycosphingolipids isolated from Aspergillus fumigatus grown in media supplemented with human serum from healthy donors. Fractionation of Cetavlon-precipitated polysaccharides on Sephacryl S-400 gave rise to an excluded fraction (Fraction I) with molecular weight of > 400 kDa and an included peak (Fraction II) with an average molecular weight of 30-80 kDa. Fraction I comprises about 5% of total polysaccharide and was identified as a glycogen-like molecule. Its structure was deduced from methylation data, treatment with amyloglucosidase, a red-brown coloration produced with an iodine solution and by 1H and 13C-NMR spectroscopy. It was previously suggested that higher amounts of glycogen-like polysaccharide (20%) were present in A. fumigatus grown in serum-free medium. Fraction II was identified as a galactomannan and was the main polysaccharide of A. fumigatus grown in serum-free medium. Fraction II was identified as a galactomannan and was the main 13C-NMR spectroscopy combined with partial acetolysis and methylation analysis. The 13C-NMR spectrum of the galactomannan showed a much greater complexity in the beta-D-gal f and alpha-D-man p C-1 regions, than was evident for galactomannan from serum-free cultures previously described, reflecting differences in the glycosylation pattern, stimulated in serum-supplemented medium. No differences in A. fumigatus glycosphingolipid could be detected between serum-containing and serum-free growth conditions. Our results demonstrate that the change in polysaccharide structure is a more specific response to the altered growth conditions and not merely a symptom of more general changes.

Publication types

  • Research Support, Non-U.S. Gov't

MeSH terms

  • Aspergillus fumigatus / chemistry*
  • Aspergillus fumigatus / growth & development
  • Blood
  • Carbohydrate Sequence
  • Culture Media
  • Galactose / analogs & derivatives
  • Glucans / chemistry
  • Glycogen / chemistry
  • Glycosphingolipids / chemistry*
  • Humans
  • Magnetic Resonance Spectroscopy
  • Mannans / chemistry
  • Methylation
  • Molecular Sequence Data
  • Polysaccharides / chemistry*
  • Spectrometry, Mass, Fast Atom Bombardment

Substances

  • Culture Media
  • Glucans
  • Glycosphingolipids
  • Mannans
  • Polysaccharides
  • galactomannan
  • Glycogen
  • Galactose