Improved quantification of 8-epi-prostaglandin F2 alpha and F2-isoprostanes by gas chromatography/triple-stage quadrupole mass spectrometry: partial cyclooxygenase-dependent formation of 8-epi-prostaglandin F2 alpha in humans

J Mass Spectrom. 1997 Dec;32(12):1362-70. doi: 10.1002/(SICI)1096-9888(199712)32:12<1362::AID-JMS606>3.0.CO;2-N.

Abstract

F2-isoprostanes are considered to be novel markers of lipid peroxidation. To study the in vivo formation of F2-isoprostanes, an improved method was developed for isotope dilution assays involving gas chromatography/triple-stage quadrupole mass spectrometry (GC/MS/MS) including thin-layer chromatography (TLC) (sum of all F2-isoprostanes) and high-performance liquid chromatographic (HPLC) purification (prostaglandin F2 alpha (PGF2 alpha) and 8-epi-PGF2 alpha). Following the addition of isotopically labeled prostaglandins to urine, the sample was acidified and applied to a C18 cartridge. After elution, prostaglandins were derivatized to pentafluorobenzyl esters and subjected to TLC. A broad zone was scratched off, isoprostanes were eluted and after formation of their trimethylsilyl ether derivatives the sum of F2-isoprostanes was determined by GC/MS/MS. For the determination of PGE2 alpha and 8-epi-PGF2 alpha prior to trimethylsilylation an additional HPLC step was performed and the fractions containing PGF2 alpha and 8-epi-PGF2 alpha were analyzed by GC/MS/MS. Using this technique, 8-epi-PGF2 alpha concentrations in urine samples as low as 5 pg ml-1 could be determined with high accuracy. The excretion rates of isoprostanes were studied in comparison with the classical prostaglandins in three different groups: healthy adults, healthy children and children with hyper-PGE syndrome (HPS), a pathological situation associated with a stimulated PGE2 synthesis. F2-isoprostanes represented the main arachidonic acid metabolites in these groups and 8-epi-PGF2 alpha excretion was comparable in its amount to the classical prostanoids. To delineate the cyclooxygenase-catalyzed contribution, the influence of indomethacin, an inhibitor of cyclooxygenases, on F2-isoprostane formation in healthy adults and in HPS children was analyzed. Significantly decreased excretion rates were observed 2 days after indomethacin administration for all prostanoids, including F2-isoprostanes and 8-epi-PGF2 alpha. However, the suppression of F2-isoprostanes and 8-epi-PGF2 alpha excretion rates was less pronounced in comparison with the classical prostanoids. An improved and reliable method for the determination of F2-isoprostanes and especially 8-epi-PGF2 alpha has been developed. The data obtained on human urine samples indicates a contribution of the cyclooxygenase pathway to the formation of isoprostanes.

Publication types

  • Clinical Trial

MeSH terms

  • Adolescent
  • Adult
  • Child
  • Chromatography, High Pressure Liquid
  • Chromatography, Thin Layer
  • Cyclooxygenase Inhibitors / therapeutic use
  • Dinoprost / analogs & derivatives*
  • Dinoprost / analysis
  • Dinoprost / biosynthesis
  • Dinoprost / urine
  • Electrophoresis, Polyacrylamide Gel
  • F2-Isoprostanes
  • Female
  • Gas Chromatography-Mass Spectrometry
  • Humans
  • Indicators and Reagents
  • Indomethacin / therapeutic use
  • Male
  • Metabolism, Inborn Errors / drug therapy
  • Metabolism, Inborn Errors / urine
  • Prostaglandin-Endoperoxide Synthases / metabolism*
  • Reference Values

Substances

  • Cyclooxygenase Inhibitors
  • F2-Isoprostanes
  • Indicators and Reagents
  • 8-epi-prostaglandin F2alpha
  • Dinoprost
  • Prostaglandin-Endoperoxide Synthases
  • Indomethacin