Cloning, sequence and expression of a linear plasmid-based and a chromosomal homolog of chloroacetaldehyde dehydrogenase-encoding genes in Xanthobacter autotrophicus GJ10

Gene. 1998 Jan 19;207(1):9-18. doi: 10.1016/s0378-1119(97)00598-2.

Abstract

The degradation of 1,2-dichloroethane (DCE) by Xanthobacter autotrophicus GJ10 proceeds via chloroacetaldehyde (CAA), a toxic intermediate in the cells if it is not metabolized further by the NAD(+)-dependent CAA dehydrogenases. Here, we describe the cloning, sequence and expression in Escherichia coli of aldA, a plasmid-located CAA dehydrogenase-encoding gene of GJ10 as well as a chromosomal homolog, designated aldB. The DNA-predicted amino acid (aa) sequences of the two proteins (505 aa in AldA and 506 aa in AldB) are 84% identical. The cloned aldA and aldB genes were verified by their expression in the E. coli T7 polymerase/promoter and the pUC lac promoter systems. The expression level of AldA and its enzymatic activity towards CAA were both higher than those of AldB. In a hybrid construct, the 3'end of aldB was able to complement, although not completely, the corresponding portion of aldA to produce a functional gene. Both AldA and AldB proteins of GJ10 share the highest degree of sequence identity with an acetaldehyde dehydrogenase (ALDH) encoded by acoD of Alcaligenes eutrophus (77.3-78% identity). Together with at least three other ALDHs of prokaryotic origin, these proteins apparently form a special class of ALDHs whose expressions are dependent on RpoN factors. By pulsed-field gel electrophoresis the 225-kb pXAU1 plasmid encoding aldA was shown to be linear.

MeSH terms

  • Acetaldehyde / analogs & derivatives
  • Acetaldehyde / metabolism
  • Aldehyde Dehydrogenase / genetics*
  • Amino Acid Sequence
  • Base Sequence
  • Biodegradation, Environmental
  • Carboxy-Lyases / genetics*
  • Cloning, Molecular
  • Escherichia coli / genetics
  • Gene Expression
  • Genes, Bacterial
  • Gram-Negative Aerobic Rods and Cocci / genetics*
  • Molecular Sequence Data
  • Plasmids
  • Promoter Regions, Genetic

Substances

  • chloroacetaldehyde
  • Aldehyde Dehydrogenase
  • Carboxy-Lyases
  • acetolactate decarboxylase
  • Acetaldehyde

Associated data

  • GENBANK/AF029733
  • GENBANK/AF029734