Analysis of oxyhalides in water by ion chromatography-ionspray mass spectrometry

J Chromatogr A. 1998 Apr 24;804(1-2):105-11. doi: 10.1016/s0021-9673(97)01244-2.

Abstract

A sensitive method for analyzing chlorite, chlorate, bromate and iodate in water by ion chromatography (IC) coupled with ionspray tandem mass spectrometry (IS-MS-MS) has been developed. Prior to analysis, samples were subjected to off-line sample clean-up with Ba, Ag and H-form resins to remove sulfate, chloride and hydrogencarbonate, respectively. Oxyhalides in the purified samples were concentrated and separated on a short, high-performance anion-exchange column. An eluent consisting of ammonium nitrate in methanol-water (9:1, v/v) was found to be suitable for separating the analytes, while providing enhanced detector sensitivity. The coupling of IC with IS-MS-MS allows for the identification of the four oxyhalides mentioned above in a single run with very high specificity and sensitivity.

Publication types

  • Comparative Study

MeSH terms

  • Drinking
  • Halogens / analysis*
  • Halogens / chemistry
  • Mass Spectrometry / methods*
  • Methanol / chemistry
  • Sensitivity and Specificity
  • Water / chemistry*

Substances

  • Halogens
  • Water
  • Methanol