All three acyl moieties of trilinolein are efficiently oxygenated by recombinant His-tagged lipid body lipoxygenase in vitro

FEBS Lett. 1998 Jul 24;431(3):433-6. doi: 10.1016/s0014-5793(98)00808-4.

Abstract

Recently, we found a 13-lipoxygenase in germinating cucumber cotyledons, which was located at the lipid body membrane. Based on its products formed mobilization of storage lipids seems to be initiated by this 13-lipoxygenase. For biochemical characterization its cDNA was expressed as His-tagged protein. Active recombinant enzyme was obtained from low temperature cultivation of E. coli after affinity purification. It (i) exhibited an unchanged region specificity, and (ii) showed a pH optimum of 7.2 against trilinolein as substrate. We compared its ability to oxygenate trilinolein with the one of another 13-lipoxygenase, soybean lipoxygenase-1. At the pH optimum of soybean lipoxygenase-1 (9.0), trilinolein was oxygenated only to 28% of the amount converted by the lipid body lipoxygenase. Moreover, trilinolein oxygenation by soybean lipoxygenase-1 leads mainly to monohydroperoxy derivatives, whereas oxygenation by lipid body LOX leads to a trihydroperoxy derivative.

Publication types

  • Research Support, Non-U.S. Gov't

MeSH terms

  • Chromatography, Affinity
  • DNA, Complementary
  • Glycine max / enzymology
  • Histidine / chemistry*
  • Hydrogen-Ion Concentration
  • Lipoxygenase / chemistry
  • Lipoxygenase / genetics
  • Lipoxygenase / metabolism*
  • Oxygen / metabolism*
  • Recombinant Proteins / metabolism
  • Substrate Specificity
  • Triglycerides / metabolism*

Substances

  • DNA, Complementary
  • Recombinant Proteins
  • Triglycerides
  • Histidine
  • Lipoxygenase
  • Oxygen
  • trilinolein