Application of lipase-catalyzed regioselective esterification in the preparation of digitonin derivatives

J Nat Prod. 1999 May;62(5):670-3. doi: 10.1021/np9803068.

Abstract

The oligosaccharide chain of the monodesmosidic haemolytic saponin digitonin (1) undergoes an efficient and regioselective acylation in organic solvent by use of Novozym 435 (lipase B from Candida antarctica supported on acrylic resin) in the presence of an activated ester. With vinyl acetate, acetylation occurs at C-6 OH of glucose(II) and C-4 OH of xylose to afford the previously unreported diacetyl derivative 2 and the monoacetyl derivatives 3 and 4. With vinyl laurate only the monolauryl derivative 5 is formed. The structures of these acylated digitonins have been established using modern 2D NMR techniques, which allowed complete assignments of all proton resonances. The hemolytic activity of derivatives 2-5 is significantly reduced compared to that of digitonin.

Publication types

  • Research Support, Non-U.S. Gov't

MeSH terms

  • Animals
  • Candida / enzymology
  • Carbohydrate Sequence
  • Cattle
  • Digitonin / analogs & derivatives*
  • Digitonin / chemical synthesis*
  • Digitonin / pharmacology
  • Esters
  • Hemolysis
  • In Vitro Techniques
  • Lipase*
  • Magnetic Resonance Spectroscopy
  • Molecular Sequence Data

Substances

  • Esters
  • Lipase
  • Digitonin